Bonding in M(NHBMe)2 and M[Mn(CO)5]2 complexes (M=Zn, Cd, Hg; NHBMe=(HCNMe)2B): divalent group 12 metals with zero oxidation state

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Varying coordination modes of amide ligand in group 12 Hg(II) and Cd(II) complexes: synthesis, crystal structure and nonlinear optical properties.

Reactions of the amide ligand, H2L (H2L = N,N'-bis[2-(2-pyridyl)methyl]pyridine-2,6-dicarboxamide) with CdCl2 and Hg(CH3COO)2, in 1 : 1 ratio, at 298 K yield dimeric [Hg(L)]2 (1) and trimeric [Cd3(H2L)4Cl6] (2), respectively. In 1, the H2L is coordinated to Hg(II) via six N-atoms of central and terminal pyridines as well as of deprotonated amido groups, whereas the carbonyl groups remain free. ...

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ژورنال

عنوان ژورنال: Theoretical Chemistry Accounts

سال: 2021

ISSN: 1432-881X,1432-2234

DOI: 10.1007/s00214-021-02751-y